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For a negative uniaxial crystal (as given in the question since n < no), the phase matching condition is given by, where, θΡΜ is the phase matching angle with respect to the optic axis of the system Now, as given, no(Zw)-1.5245, ne(2ω)-1.4802, no(W)-1.5019, ne(w)-1.4637 So, (1.5019)2(1.5245)2 sin2 θΡΜ 2 1.480221.5245 sin2 θΡΜ-0.4991 sin θΡΜ-0.7065
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